Investigating HALocarbon impacts on the global Environment (InHALE)

调查 HALocarbon 对全球环境的影响 (InHALE)

• 批准号: NE/X00452X/1
• 负责人: Matthew Rigby
• 金额: $ 247.04万
• 依托单位: University of Bristol
• 依托单位国家: 英国
• 项目类别: Research Grant
• 财政年份: 2022
• 资助国家: 英国
• 起止时间: 2022 至 无数据
• 项目状态: 未结题
• 来源: https://gtr.ukri.org/projects?ref=NE%2FX00452X%2F1
• 关键词: Investigating; HALocarbon; impacts; global; Environment

With the Kigali Amendment coming into force in 2019, the Montreal Protocol on Substances that Deplete the Ozone Layer has entered a major new phase in which the production and use of hydrofluorocarbons (HFCs) will be controlled in most major economies. This landmark achievement will enhance the Protocol's already-substantial benefits to climate, in addition to its success in protecting the ozone layer. However, recent scientific advances have shown that challenges lie ahead for the Montreal Protocol, due to the newly discovered production of ozone-depleting substances (ODS) thought to be phased-out, rapid growth of ozone-depleting compounds not controlled under the Protocol, and the potential for damaging impacts of halocarbon degradation products. This proposal tackles the most urgent scientific questions surrounding these challenges by combining state-of-the-art techniques in atmospheric measurements, laboratory experiments and advanced numerical modelling. We will: 1) significantly expand atmospheric measurement coverage to better understand the global distribution of halocarbon emissions and to identify previously unknown atmospheric trends, 2) combine industry models and atmospheric data to improve our understanding of the relationship between production (the quantity controlled under the Protocol), "banks" of halocarbons stored in buildings and products, and emissions to the atmosphere, 3) determine recent and likely future trends of unregulated, short-lived halocarbons, and implications for the timescale of recovery of the ozone layer, 4) explore the complex atmospheric chemistry of the newest generation of halocarbons and determine whether breakdown products have the potential to contribute to climate change or lead to unforeseen negative environmental consequences, 5) better quantify the influence of halocarbons on climate and refine the climate- and ozone-depletion-related metrics used to compare the effects of halocarbons in international agreements and in the design of possible mitigation strategies. This work will be carried out by a consortium of leaders in the field of halocarbon research, who have an extensive track record of contributing to Montreal Protocol bodies and the Intergovernmental Panel on Climate Change, ensuring lasting impact of the new developments that will be made.

随着《基加利修正案》于2019年生效，《关于消耗臭氧层物质的蒙特利尔议定书》进入了一个重要的新阶段，大多数主要经济体将控制氢氟碳化物（HFC）的生产和使用。这一具有里程碑意义的成就除了在保护臭氧层方面取得的成功之外，还将增强该议定书对气候已有的实质性效益。然而，最近的科学进展表明，《蒙特利尔议定书》面临着挑战，因为新发现的臭氧消耗物质（ODS）的生产被认为已被逐步淘汰，而不受《议定书》控制的臭氧消耗化合物的快速增长，以及卤化碳降解产物的潜在破坏性影响。该提案通过结合大气测量、实验室实验和先进数值建模领域的最先进技术，解决了围绕这些挑战的最紧迫的科学问题。我们将：1）显着扩大大气测量覆盖范围，以更好地了解卤化碳排放的全球分布，并识别以前未知的大气趋势，2）结合行业模型和大气数据，以提高我们对生产（在控制下控制的数量）之间关系的理解。议定书），储存在建筑物和产品中的卤化碳“库”，以及向大气的排放，3）确定不受管制的短期卤化碳的近期和可能的未来趋势，以及对臭氧层恢复时间尺度的影响，4）探索最新一代卤化碳的复杂大气化学性质，并确定分解产物是否有可能导致气候变化或导致不可预见的负面环境后果，5) 更好地量化卤化碳对气候的影响，并完善气候和臭氧消耗- 用于比较卤代碳在国际协议和可能的缓解战略设计中的影响的相关指标。这项工作将由卤碳研究领域的领导者联盟进行，他们在为《蒙特利尔议定书》机构和政府间气候变化专门委员会做出贡献方面有着广泛的记录，确保将要取得的新进展产生持久影响。

项目成果

Global increase of ozone-depleting chlorofluorocarbons from 2010 to 2020

2010年至2020年全球消耗臭氧层氯氟烃的增加

• DOI: 10.1038/s41561-023-01147-w
• 发表时间: 2023-04-01
• 期刊: Nature Geoscience
• 影响因子: 18.3
• 作者: L. Western;M. Vollmer;P. Krummel;Karina E. Adcock;M. Crotwell;P. Fraser;C. Harth;R. Langenfelds;S. Montzka;Jens Mühle;S. O'Doherty;D. Oram;S. Reimann;M. Rigby;I. Vimont;R. Weiss;D. Young;J. Laube
• 通讯作者: J. Laube

Author Correction: Global increase of ozone-depleting chlorofluorocarbons from 2010 to 2020

作者更正：2010年至2020年全球消耗臭氧层氯氟碳化合物增加

• DOI: http://dx.10.1038/s41561-023-01205-3
• 发表时间: 2023
• 期刊: Nature Geoscience
• 影响因子: 18.3
• 作者: Western L

In Situ Observations of Halogenated Gases at the Shangdianzi Background Station and Emission Estimates for Northern China

上甸子背景站卤化气体现场观测及华北地区排放估算

• DOI: http://dx.10.1021/acs.est.3c00695
• 发表时间: 2023
• 期刊: Environmental Science & Technology
• 影响因子: 11.4
• 作者: Yi L

Anthropogenic Chloroform Emissions from China Drive Changes in Global Emissions

中国人为氯仿排放推动全球排放变化

• DOI: http://dx.10.1021/acs.est.3c01898
• 发表时间: 2023
• 期刊: Environmental Science & Technology
• 影响因子: 11.4
• 作者: An M