CAREER: Fundamental Investigation of the Wave Nature of Lattice Thermal Transport

职业：晶格热传输波性质的基础研究

• 批准号: 2047109
• 负责人: Yan Wang
• 金额: $ 51.21万
• 依托单位: Board of Regents, NSHE, obo University of Nevada, Reno
• 依托单位国家: 美国
• 项目类别: Continuing Grant
• 财政年份: 2021
• 资助国家: 美国
• 起止时间: 2021-07-01 至 2026-12-31
• 项目状态: 未结题
• 来源: https://www.nsf.gov/awardsearch/showAward?AWD_ID=2047109&HistoricalAwards=false
• 关键词: CAREER; Fundamental; Investigation; Wave; Nature

Heat transfer is a limiting factor in nanoscale engineering: if the finely tuned elements such as microchips or lasers get too hot or conduct heat uncontrollably, the devices will not function as intended. Thus, understanding how to control heat transfer at the nanoscale is critical in many engineering applications. Heat conduction in semiconductor crystals is dominated by collective atomic vibrations known as phonons. Conventionally, phonons are treated as particles that can propagate through a material, thus carrying heat, and can be scattered by material defects or other phonons. However, the wave nature of phonons can emerge or even dominate heat conduction in structures composed of periodically or quasi-periodically arranged components, e.g., quantum cascade lasers made of alternating layers of materials and integrated circuits containing densely packed nano-transistors. In those structures, the propagation of phonons can be promoted by constructive interference or halted by destructive interference. This project aims to explore these intriguing wave behaviors and elucidate the transition between particle-like and wave-like phonons through complementary computational and experimental techniques. This research will lead to novel engineering strategies to maximize heat dissipation in modern devices like quantum cascade lasers and integrated circuits or minimize heat conduction in thermoelectric materials and thermal barriers. This project will tightly integrate research, education, and outreach—including themed science exhibits, new curriculum development, hands-on research mentoring, and online course and research tool sharing—to have a broad, long-term impact on STEM education for K-12, undergraduate, and graduate students. The research objectives of this project are to: 1) rigorously understand the transport, scattering, and localization of wave-like phonons in periodic, quasi-periodic, and aperiodic structures, leveraging complementary spectral phonon analysis and phonon spectroscopy techniques; and 2) minimize lattice thermal transport through decoupled suppression of wave-like and particle-like phonon transport, leveraging machine learning-aided spectral phonon analysis and structure optimization. The proposed research on the wave nature of phonons can greatly advance the state of knowledge of thermal transport in crystalline solids, which has until now been primarily based on the particle nature of phonons. Such knowledge will enable the development of novel engineering strategies based on the wave nature of phonons, breaking the bottleneck of the thermal design or management of various heat transfer-limited technologies.This award reflects NSF's statutory mission and has been deemed worthy of support through evaluation using the Foundation's intellectual merit and broader impacts review criteria.

传热是纳米级工程的一个限制因素：如果微芯片或激光器等微调元件变得太热或无法控制地传导热量，设备将无法按预期工作，因此，了解如何控制纳米级传热至关重要。在许多工程应用中，半导体晶体中的热传导主要由称为声子的集体原子振动主导，声子被视为可以在材料中传播的粒子，从而携带热量，并且可以因材料缺陷或其他原因而散射。然而，声子的波性质可以在由周期性或准周期性排列的部件组成的结构中出现甚至主导热传导，例如由交替的材料层和包含密集纳米晶体管的集成电路制成的量子级联激光器。在这些结构中，声子的传播可以通过相长干涉来促进或通过相消干涉来停止。该项目旨在探索这些有趣的波行为并阐明粒子状和波状之间的转变。该研究将通过互补的计算和实验技术产生新颖的工程策略，以最大限度地提高量子级联激光器和集成电路等现代设备的散热能力，或最大限度地减少热电材料和热屏障中的热传导。和推广——包括主题科学展览、新课程开发、实践研究指导以及在线课程和研究工具共享——对 K-12、本科生和研究生的 STEM 教育产生广泛、长期的影响。目标该项目的目标是：1）利用互补光谱声子分析和声子光谱技术，严格了解周期性、准周期性和非周期性结构中波状声子的输运、散射和局域化；2）最大限度地减少晶格热输运；通过波状和粒子状声子输运的解耦抑制，利用机器学习辅助的谱声子分析和结构优化。声子的波性质可以极大地推进晶体固体热传输的知识状态，迄今为止，这种知识主要基于声子的粒子性质，这些知识将使基于声子的波性质的新颖工程策略的开发成为可能。打破各种传热限制技术的热设计或管理瓶颈。该奖项反映了 NSF 的法定使命，并通过使用基金会的智力价值和更广泛的影响审查标准进行评估，被认为值得支持。

项目成果

Lattice thermal conductivity of embedded nanoparticle composites: the role of particle size distribution

嵌入纳米粒子复合材料的晶格热导率：粒度分布的作用

• DOI: 10.1088/1361-6528/ad06d6
• 发表时间: 2023-11-15
• 期刊: Nanotechnology
• 影响因子: 3.5
• 作者: Theodore Maranets;Haoran Cui;Yan Wang
• 通讯作者: Yan Wang

Ballistic phonon lensing by the non-planar interfaces of embedded nanoparticles

嵌入纳米粒子的非平面界面的弹道声子透镜

• DOI: 10.1088/1367-2630/ad025a
• 发表时间: 2023-10-01
• 期刊: New Journal of Physics
• 影响因子: 3.3
• 作者: Theodore Maranets;Yan Wang
• 通讯作者: Yan Wang

Ex-situ modification of lattice thermal transport through coherent and incoherent heat baths

通过相干和非相干热浴对晶格热传输进行异位修改

• DOI: 10.1016/j.mtphys.2022.100884
• 发表时间: 2022-10-01
• 期刊: Materials Today Physics
• 影响因子: 11.5
• 作者: Tengfei Ma;Yan Wang
• 通讯作者: Yan Wang